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Intercontinental transport of anthropogenic sulfur dioxide and other pollutants: An infrared remote sensing case study

Identifieur interne : 000009 ( PascalFrancis/Corpus ); précédent : 000008; suivant : 000010

Intercontinental transport of anthropogenic sulfur dioxide and other pollutants: An infrared remote sensing case study

Auteurs : Lieven Clarisse ; Michael Fromm ; Yasmine Ngadi ; Louisa Emmons ; Cathy Clerbaux ; Daniel Hurtmans ; Pierre-François Coheur

Source :

RBID : Pascal:14-0045125

Descripteurs français

English descriptors

Abstract

[1] Using 3 years worth of IASI (the Infrared Atmospheric Sounder Interferometer aboard METOP-A) measurements, we have identified 24 major events of uplift and transport of anthropogenic sulfur dioxide. These were all first observed over East Asia, and could be traced for over 60 hours. On 7 November 2010 a sulfur dioxide plume was observed over Northeast China and tracked for five days to North America. We discuss this event in detail with respect to build up; uplift and in-plume chemistry. We found a host of trace gas enhancements in the plume (SO2, CO, PAN, CH3OH, HCOOH and C2H2). A reasonable to very good agreement was found with MOZART-4 modeled ambient columns for all species except methanol, which was underestimated by the model by an order of magnitude. We calculate correlations of the different species and give observational evidence of secondary in-plume formation of methanol and PAN.

Notice en format standard (ISO 2709)

Pour connaître la documentation sur le format Inist Standard.

pA  
A01 01  1    @0 0094-8276
A02 01      @0 GPRLAJ
A03   1    @0 Geophys. res. lett.
A05       @2 38
A06       @2 19
A08 01  1  ENG  @1 Intercontinental transport of anthropogenic sulfur dioxide and other pollutants: An infrared remote sensing case study
A11 01  1    @1 CLARISSE (Lieven)
A11 02  1    @1 FROMM (Michael)
A11 03  1    @1 NGADI (Yasmine)
A11 04  1    @1 EMMONS (Louisa)
A11 05  1    @1 CLERBAUX (Cathy)
A11 06  1    @1 HURTMANS (Daniel)
A11 07  1    @1 COHEUR (Pierre-François)
A14 01      @1 Spectroscopie de l'Atmosphère, Service de Chimie Quantique et Photophysique, Université Libre de Bruxelles @2 Brussels @3 BEL @Z 1 aut. @Z 3 aut. @Z 5 aut. @Z 6 aut. @Z 7 aut.
A14 02      @1 U.S. Naval Research Laboratory @2 Washington, DC @3 USA @Z 2 aut.
A14 03      @1 National Center for Atmospheric Research @2 Boulder, Colorado @3 USA @Z 4 aut.
A14 04      @1 UPMC Université Paris 6, Université Versailles St.-Quentin, CNRS/INSU, LATMOS-IPSL @2 Paris @3 FRA @Z 5 aut.
A20       @2 L19806.1-L19806.5
A21       @1 2011
A23 01      @0 ENG
A43 01      @1 INIST @2 16687 @5 354000501660740490
A44       @0 0000 @1 © 2014 INIST-CNRS. All rights reserved.
A45       @0 3/4 p.
A47 01  1    @0 14-0045125
A60       @1 P
A61       @0 A
A64 01  1    @0 Geophysical research letters
A66 01      @0 USA
C01 01    ENG  @0 [1] Using 3 years worth of IASI (the Infrared Atmospheric Sounder Interferometer aboard METOP-A) measurements, we have identified 24 major events of uplift and transport of anthropogenic sulfur dioxide. These were all first observed over East Asia, and could be traced for over 60 hours. On 7 November 2010 a sulfur dioxide plume was observed over Northeast China and tracked for five days to North America. We discuss this event in detail with respect to build up; uplift and in-plume chemistry. We found a host of trace gas enhancements in the plume (SO2, CO, PAN, CH3OH, HCOOH and C2H2). A reasonable to very good agreement was found with MOZART-4 modeled ambient columns for all species except methanol, which was underestimated by the model by an order of magnitude. We calculate correlations of the different species and give observational evidence of secondary in-plume formation of methanol and PAN.
C02 01  3    @0 001E
C02 02  2    @0 001E01
C02 03  2    @0 220
C03 01  2  FRE  @0 Transport @5 01
C03 01  2  ENG  @0 transport @5 01
C03 01  2  SPA  @0 Transporte @5 01
C03 02  X  FRE  @0 Facteur anthropique @5 02
C03 02  X  ENG  @0 Anthropogenic factor @5 02
C03 02  X  SPA  @0 Factor antrópico @5 02
C03 03  2  FRE  @0 Dioxyde soufre @5 03
C03 03  2  ENG  @0 sulfur dioxide @5 03
C03 04  X  FRE  @0 Dioxyde de soufre @2 NK @2 FX @5 04
C03 04  X  ENG  @0 Sulfur dioxide @2 NK @2 FX @5 04
C03 04  X  SPA  @0 Dióxido sulfúrico @2 NK @2 FX @5 04
C03 05  2  FRE  @0 Polluant @5 05
C03 05  2  ENG  @0 pollutants @5 05
C03 05  2  SPA  @0 Contaminante @5 05
C03 06  2  FRE  @0 Télédétection spatiale @5 06
C03 06  2  ENG  @0 Space remote sensing @5 06
C03 06  2  SPA  @0 Teledetección espacial @5 06
C03 07  2  FRE  @0 Etude cas @5 07
C03 07  2  ENG  @0 case studies @5 07
C03 07  2  SPA  @0 Estudio caso @5 07
C03 08  2  FRE  @0 Surrection @5 08
C03 08  2  ENG  @0 uplifts @5 08
C03 09  2  FRE  @0 Panache @5 09
C03 09  2  ENG  @0 plumes @5 09
C03 09  2  SPA  @0 Penacho @5 09
C03 10  2  FRE  @0 Trajectoire @5 10
C03 10  2  ENG  @0 trajectory @5 10
C03 11  2  FRE  @0 Amérique du Nord @5 11
C03 11  2  ENG  @0 North America @5 11
C03 11  2  SPA  @0 America del norte @5 11
C03 12  X  FRE  @0 Composé trace @5 12
C03 12  X  ENG  @0 Trace compound @5 12
C03 12  X  SPA  @0 Compuesto huella @5 12
C03 13  X  FRE  @0 Pan @2 NO @5 13
C03 13  X  ENG  @0 Pan @2 NO @5 13
C03 13  X  SPA  @0 Pan @2 NO @5 13
C03 14  X  FRE  @0 Méthanol @2 NK @2 FX @5 14
C03 14  X  ENG  @0 Methanol @2 NK @2 FX @5 14
C03 14  X  SPA  @0 Metanol @2 NK @2 FX @5 14
C03 15  2  FRE  @0 Modèle @5 15
C03 15  2  ENG  @0 models @5 15
C03 15  2  SPA  @0 Modelo @5 15
C03 16  2  FRE  @0 Corrélation @5 16
C03 16  2  ENG  @0 correlation @5 16
C03 16  2  SPA  @0 Correlación @5 16
C03 17  X  FRE  @0 Observation par satellite @5 17
C03 17  X  ENG  @0 Satellite observation @5 17
C03 17  X  SPA  @0 Observación por satélite @5 17
C03 18  2  FRE  @0 Chine @2 NG @5 61
C03 18  2  ENG  @0 China @2 NG @5 61
C03 18  2  SPA  @0 China @2 NG @5 61
C07 01  2  FRE  @0 Extrême Orient @2 NG
C07 01  2  ENG  @0 Far East @2 NG
C07 01  2  SPA  @0 Extremo Oriente @2 NG
C07 02  2  FRE  @0 Asie @2 564
C07 02  2  ENG  @0 Asia @2 564
C07 02  2  SPA  @0 Asia @2 564
N21       @1 055
N44 01      @1 OTO
N82       @1 OTO

Format Inist (serveur)

NO : PASCAL 14-0045125 INIST
ET : Intercontinental transport of anthropogenic sulfur dioxide and other pollutants: An infrared remote sensing case study
AU : CLARISSE (Lieven); FROMM (Michael); NGADI (Yasmine); EMMONS (Louisa); CLERBAUX (Cathy); HURTMANS (Daniel); COHEUR (Pierre-François)
AF : Spectroscopie de l'Atmosphère, Service de Chimie Quantique et Photophysique, Université Libre de Bruxelles/Brussels/Belgique (1 aut., 3 aut., 5 aut., 6 aut., 7 aut.); U.S. Naval Research Laboratory/Washington, DC/Etats-Unis (2 aut.); National Center for Atmospheric Research/Boulder, Colorado/Etats-Unis (4 aut.); UPMC Université Paris 6, Université Versailles St.-Quentin, CNRS/INSU, LATMOS-IPSL/Paris/France (5 aut.)
DT : Publication en série; Niveau analytique
SO : Geophysical research letters; ISSN 0094-8276; Coden GPRLAJ; Etats-Unis; Da. 2011; Vol. 38; No. 19; L19806.1-L19806.5; Bibl. 3/4 p.
LA : Anglais
EA : [1] Using 3 years worth of IASI (the Infrared Atmospheric Sounder Interferometer aboard METOP-A) measurements, we have identified 24 major events of uplift and transport of anthropogenic sulfur dioxide. These were all first observed over East Asia, and could be traced for over 60 hours. On 7 November 2010 a sulfur dioxide plume was observed over Northeast China and tracked for five days to North America. We discuss this event in detail with respect to build up; uplift and in-plume chemistry. We found a host of trace gas enhancements in the plume (SO2, CO, PAN, CH3OH, HCOOH and C2H2). A reasonable to very good agreement was found with MOZART-4 modeled ambient columns for all species except methanol, which was underestimated by the model by an order of magnitude. We calculate correlations of the different species and give observational evidence of secondary in-plume formation of methanol and PAN.
CC : 001E; 001E01; 220
FD : Transport; Facteur anthropique; Dioxyde soufre; Dioxyde de soufre; Polluant; Télédétection spatiale; Etude cas; Surrection; Panache; Trajectoire; Amérique du Nord; Composé trace; Pan; Méthanol; Modèle; Corrélation; Observation par satellite; Chine
FG : Extrême Orient; Asie
ED : transport; Anthropogenic factor; sulfur dioxide; Sulfur dioxide; pollutants; Space remote sensing; case studies; uplifts; plumes; trajectory; North America; Trace compound; Pan; Methanol; models; correlation; Satellite observation; China
EG : Far East; Asia
SD : Transporte; Factor antrópico; Dióxido sulfúrico; Contaminante; Teledetección espacial; Estudio caso; Penacho; America del norte; Compuesto huella; Pan; Metanol; Modelo; Correlación; Observación por satélite; China
LO : INIST-16687.354000501660740490
ID : 14-0045125

Links to Exploration step

Pascal:14-0045125

Le document en format XML

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<term>Transport</term>
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<term>Surrection</term>
<term>Panache</term>
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<term>Composé trace</term>
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<div type="abstract" xml:lang="en">[1] Using 3 years worth of IASI (the Infrared Atmospheric Sounder Interferometer aboard METOP-A) measurements, we have identified 24 major events of uplift and transport of anthropogenic sulfur dioxide. These were all first observed over East Asia, and could be traced for over 60 hours. On 7 November 2010 a sulfur dioxide plume was observed over Northeast China and tracked for five days to North America. We discuss this event in detail with respect to build up; uplift and in-plume chemistry. We found a host of trace gas enhancements in the plume (SO
<sub>2</sub>
, CO, PAN, CH
<sub>3</sub>
OH, HCOOH and C
<sub>2</sub>
H
<sub>2</sub>
). A reasonable to very good agreement was found with MOZART-4 modeled ambient columns for all species except methanol, which was underestimated by the model by an order of magnitude. We calculate correlations of the different species and give observational evidence of secondary in-plume formation of methanol and PAN.</div>
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<s1>U.S. Naval Research Laboratory</s1>
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<s1>National Center for Atmospheric Research</s1>
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<s0>[1] Using 3 years worth of IASI (the Infrared Atmospheric Sounder Interferometer aboard METOP-A) measurements, we have identified 24 major events of uplift and transport of anthropogenic sulfur dioxide. These were all first observed over East Asia, and could be traced for over 60 hours. On 7 November 2010 a sulfur dioxide plume was observed over Northeast China and tracked for five days to North America. We discuss this event in detail with respect to build up; uplift and in-plume chemistry. We found a host of trace gas enhancements in the plume (SO
<sub>2</sub>
, CO, PAN, CH
<sub>3</sub>
OH, HCOOH and C
<sub>2</sub>
H
<sub>2</sub>
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<s5>04</s5>
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<s2>FX</s2>
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<s5>07</s5>
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<s5>07</s5>
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<s5>08</s5>
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<s0>uplifts</s0>
<s5>08</s5>
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<s5>09</s5>
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<s5>09</s5>
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<s5>09</s5>
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<s5>10</s5>
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<s5>10</s5>
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<s5>11</s5>
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<s5>11</s5>
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<s5>11</s5>
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<s5>12</s5>
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<fC03 i1="12" i2="X" l="ENG">
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<s5>12</s5>
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<s0>Compuesto huella</s0>
<s5>12</s5>
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<fC03 i1="13" i2="X" l="FRE">
<s0>Pan</s0>
<s2>NO</s2>
<s5>13</s5>
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<fC03 i1="13" i2="X" l="ENG">
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<s5>13</s5>
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<s5>13</s5>
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<s5>14</s5>
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<s2>FX</s2>
<s5>14</s5>
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<s5>14</s5>
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<s5>61</s5>
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<server>
<NO>PASCAL 14-0045125 INIST</NO>
<ET>Intercontinental transport of anthropogenic sulfur dioxide and other pollutants: An infrared remote sensing case study</ET>
<AU>CLARISSE (Lieven); FROMM (Michael); NGADI (Yasmine); EMMONS (Louisa); CLERBAUX (Cathy); HURTMANS (Daniel); COHEUR (Pierre-François)</AU>
<AF>Spectroscopie de l'Atmosphère, Service de Chimie Quantique et Photophysique, Université Libre de Bruxelles/Brussels/Belgique (1 aut., 3 aut., 5 aut., 6 aut., 7 aut.); U.S. Naval Research Laboratory/Washington, DC/Etats-Unis (2 aut.); National Center for Atmospheric Research/Boulder, Colorado/Etats-Unis (4 aut.); UPMC Université Paris 6, Université Versailles St.-Quentin, CNRS/INSU, LATMOS-IPSL/Paris/France (5 aut.)</AF>
<DT>Publication en série; Niveau analytique</DT>
<SO>Geophysical research letters; ISSN 0094-8276; Coden GPRLAJ; Etats-Unis; Da. 2011; Vol. 38; No. 19; L19806.1-L19806.5; Bibl. 3/4 p.</SO>
<LA>Anglais</LA>
<EA>[1] Using 3 years worth of IASI (the Infrared Atmospheric Sounder Interferometer aboard METOP-A) measurements, we have identified 24 major events of uplift and transport of anthropogenic sulfur dioxide. These were all first observed over East Asia, and could be traced for over 60 hours. On 7 November 2010 a sulfur dioxide plume was observed over Northeast China and tracked for five days to North America. We discuss this event in detail with respect to build up; uplift and in-plume chemistry. We found a host of trace gas enhancements in the plume (SO
<sub>2</sub>
, CO, PAN, CH
<sub>3</sub>
OH, HCOOH and C
<sub>2</sub>
H
<sub>2</sub>
). A reasonable to very good agreement was found with MOZART-4 modeled ambient columns for all species except methanol, which was underestimated by the model by an order of magnitude. We calculate correlations of the different species and give observational evidence of secondary in-plume formation of methanol and PAN.</EA>
<CC>001E; 001E01; 220</CC>
<FD>Transport; Facteur anthropique; Dioxyde soufre; Dioxyde de soufre; Polluant; Télédétection spatiale; Etude cas; Surrection; Panache; Trajectoire; Amérique du Nord; Composé trace; Pan; Méthanol; Modèle; Corrélation; Observation par satellite; Chine</FD>
<FG>Extrême Orient; Asie</FG>
<ED>transport; Anthropogenic factor; sulfur dioxide; Sulfur dioxide; pollutants; Space remote sensing; case studies; uplifts; plumes; trajectory; North America; Trace compound; Pan; Methanol; models; correlation; Satellite observation; China</ED>
<EG>Far East; Asia</EG>
<SD>Transporte; Factor antrópico; Dióxido sulfúrico; Contaminante; Teledetección espacial; Estudio caso; Penacho; America del norte; Compuesto huella; Pan; Metanol; Modelo; Correlación; Observación por satélite; China</SD>
<LO>INIST-16687.354000501660740490</LO>
<ID>14-0045125</ID>
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